Major Mabuzaa

Major Mabuzaa,, Kasturie Premlalla, Maurice Onyangoa, Michael O. Daramolab aDepartment of Chemical Metallurgical Engineering, Tshwane University of Technology, Private Bag X680, Pretoria, 0001, Republic of South Africa bSchool of Chemical Metallurgical Engineering, Faculty of Engineering and the Built Environment, University of the Witwatersrand, Private Bag 3, Wits 2050, Johannesburg, Republic of South Africa Corresponding Author Email HYPERLINK [email protected] [email protected] ABSTRACT There have recently been numerous research projects that focus on the reduction of carbon dioxide (CO2) emissions caused by humanity. CO2 storage in unmineable coal seams has been identified as one of the resolutions to sequester the captured CO2 while (in some cases) recovering methane (CH4). However, CO2 injected into coal seams normally contains additional gases that may well reduce the coal storage capacity, cause changes in the sorption behavior and physicochemical properties of the coal. This research aimed to investigate the sorption behavior of three South African coals (sorbents) upon pure CO2 and flue gas (sorbates) sorption. Sorption measurements were conducted on 10 g samples with a grain size passing through a 2-mm sieve. A synthetic industrial flue gas containing 12 CO2, 5.5 O2, 82 N2, 0.38 SO2, and 0.12 NO2 was used in the current study. Sorption isotherms were measured at a temperature ranging from 30 60 C and pressures up to 9.0 MPa using a High-Pressure CO2 Volumetric Adsorption System (HPCVAS). It was found that the sorption of CO2 onto coal is highly reduced by the presence of additional gases due to competition for sorption sites hence the reduction in CO2 (in flue gas) sorption capacity of coal of up to 63 compared to using pure CO2. Keywords Carbon dioxide Coal Flue gas Preferential sorption Sorption capacity Introduction Since the start of the industrial evolution, large amounts of greenhouse gases (GHGs) have been emitted by humanity into the atmosphere, these include some radioactive gases HYPERLINK l _ENREF_1 o Chiari, 2011 445 ADDIN EN.CITE EndNoteCiteAuthorChiari/AuthorYear2011/YearRecNum445/RecNumDisplayTextstyle facesuperscript1/style/DisplayTextrecordrec-number445/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp1515757404445/key/foreign-keysref-type nameJournal Article17/ref-typecontributorsauthorsauthorChiari, Luca/authorauthorZecca, Antonio/author/authors/contributorstitlestitleConstraints of fossil fuels depletion on global warming projections/titlesecondary-titleEnergy Policy/secondary-title/titlesperiodicalfull-titleEnergy Policy/full-title/periodicalpages5026-5034/pagesvolume39/volumenumber9/numberkeywordskeywordClimatic projections/keywordkeywordFossil fuels depletion/keywordkeywordEmissions scenarios/keyword/keywordsdatesyear2011/year/datesisbn0301-4215/isbnurlsrelated-urlsurlhttp//www.sciencedirect.com/science/article/pii/S0301421511004654/url/related-urls/urlselectronic-resource-numhttp//dx.doi.org/10.1016/j.enpol.2011.06.011/electronic-resource-num/record/Cite/EndNote1. This has led to climate change for which is one of the main risks currently facing humanity. The continuous burning of fossil fuel increases the atmospheric CO2 concentration year on year, contributing to greenhouse gas emissions that warm the planet. To what extent, then, must CO2 emissions be kept under control in order to restrict global temperature rise to within 2 C The link between climate change and CO2 emissions has since caught the attention of scientists, politicians, and the general public, through the renowned greenhouse effect HYPERLINK l _ENREF_2 o Lacis, 2010 442 ADDIN EN.CITE EndNoteCiteAuthorLacis/AuthorYear2010/YearRecNum442/RecNumDisplayTextstyle facesuperscript2/style/DisplayTextrecordrec-number442/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp1515757404442/key/foreign-keysref-type nameJournal Article17/ref-typecontributorsauthorsauthorLacis, Andrew A./authorauthorSchmidt, Gavin A./authorauthorRind, David/authorauthorRuedy, Reto A./author/authors/contributorstitlestitlestyle facenormal fontdefault size100Atmospheric CO/stylestyle facesubscript fontdefault size1002/stylestyle facenormal fontdefault size100 Principal Control Knob Governing Earths Temperature/style/titlesecondary-titleScience/secondary-title/titlesperiodicalfull-titleScience/full-title/periodicalpages356-359/pagesvolume330/volumenumber6002/numberdatesyear2010/year/datesurlsrelated-urlsurlhttp//science.sciencemag.org/content/sci/330/6002/356.full.pdf/url/related-urls/urlselectronic-resource-num10.1126/science.1190653/electronic-resource-num/record/Cite/EndNote2. In order to maintain the atmospheric CO2 concentrations between 450 and 650 ppm by 2100, this would require an extreme radical reduction in anthropogenic CO2 emissions over the forthcoming 20 30 years. Eventually, reducing the GHG emissions will be a supreme mitigating action, necessitating more efficient and cleaner energy sources than fossil fuels, and other changes in current humanity activities HYPERLINK l _ENREF_3 o Mandlebaum, 2011 444 ADDIN EN.CITE EndNoteCiteAuthorMandlebaum/AuthorYear2011/YearRecNum444/RecNumDisplayTextstyle facesuperscript3/style/DisplayTextrecordrec-number444/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp1515757404444/key/foreign-keysref-type nameBook Section5/ref-typecontributorsauthorsauthorMandlebaum, S./authorauthorNriagu, J./author/authors/contributorstitlestitleCarbon Sequestration and Agriculture/titlesecondary-titleEncyclopedia of Environmental Health/secondary-title/titlespages498-504/pageskeywordskeywordAgriculture/keywordkeywordAgronomic practices/keywordkeywordCapacity/keywordkeywordCarbon/keywordkeywordCarbon cycle/keywordkeywordCarbon dioxide/keywordkeywordClimate change/keywordkeywordConservation/keywordkeywordHealth/keywordkeywordSequestration/keywordkeywordSink/keywordkeywordSoil/keywordkeywordStorage/keywordkeywordTillage/keyword/keywordsdatesyear2011/year/datespub-locationBurlington/pub-locationpublisherElsevier/publisherisbn978-0-444-52272-6/isbnurlsrelated-urlsurlhttp//www.sciencedirect.com/science/article/pii/B9780444522726007339/url/related-urls/urlselectronic-resource-numhttp//dx.doi.org/10.1016/B978-0-444-52272-6.00733-9/electronic-resource-num/record/Cite/EndNote3. At the United Nations Climate Change Conference held in Paris at the end of 2015, 195 countries (including South Africa) settled on a plan to lessen the CO2 emissions and other greenhouse gases. This was aimed at limiting the global temperature to well below 2 C (this is relative to pre-industrialization evolution climate thus, future global warming should be limited to below 1.4 C since, at the end of the twentieth century, the global temperature had already increased by 0.6 C) HYPERLINK l _ENREF_4 o Anderson, 2016 441 ADDIN EN.CITE EndNoteCiteAuthorAnderson/AuthorYear2016/YearRecNum441/RecNumDisplayTextstyle facesuperscript4/style/DisplayTextrecordrec-number441/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp1515757404441/key/foreign-keysref-type nameJournal Article17/ref-typecontributorsauthorsauthorAnderson, Thomas R./authorauthorHawkins, Ed/authorauthorJones, Philip D./author/authors/contributorstitlestitlestyle facenormal fontdefault size100CO/stylestyle facesubscript fontdefault size1002/stylestyle facenormal fontdefault size100, the greenhouse effect and global warming from the pioneering work of Arrhenius and Callendar to todayaposs Earth System Models/style/titlesecondary-titleEndeavour/secondary-title/titlesperiodicalfull-titleEndeavour/full-title/periodicalpages178-187/pagesvolume40/volumenumber3/numberkeywordskeywordGreenhouse effect/keywordkeywordGlobal warming/keywordkeywordEarth System Models/keywordkeywordArrhenius/keywordkeywordCallendar/keyword/keywordsdatesyear2016/year/datesisbn0160-9327/isbnurlsrelated-urlsurlhttp//www.sciencedirect.com/science/article/pii/S0160932716300308/url/related-urls/urlselectronic-resource-numhttp//dx.doi.org/10.1016/j.endeavour.2016.07.002/electronic-resource-num/record/Cite/EndNote4. South Africa is one of the largest developing country emitters HYPERLINK l _ENREF_5 o van der Merwe, 2010 448 ADDIN EN.CITE EndNoteCiteAuthorvan der Merwe/AuthorYear2010/YearRecNum448/RecNumDisplayTextstyle facesuperscript5/style/DisplayTextrecordrec-number448/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp1515757404448/key/foreign-keysref-type nameElectronic Article43/ref-typecontributorsauthorsauthorvan der Merwe, C/author/authors/contributorstitlestitleEnergy amp Climate Change – Policy and Progress/title/titleseditionMay 2010/editiondatesyear2010/yearpub-datesdate06 October 2016/date/pub-dates/datespublisherstyle facenormal fontdefault size100ZEROCO/stylestyle facesubscript fontdefault size1002/style/publisherurlsrelated-urlsurlhttp//www.zeroco2.no/projects/south-africa/url/related-urls/urls/record/Cite/EndNote5. Due to the increasing worldwide focus on climate change, there has been an increasing awareness that South Africa needs to assume low-carbon intensive routes to avoid foreseeable social and financial penalties HYPERLINK l _ENREF_6 o Naidoo, 2009 449 ADDIN EN.CITE EndNoteCiteAuthorNaidoo/AuthorYear2009/YearRecNum449/RecNumDisplayTextstyle facesuperscript6/style/DisplayTextrecordrec-number449/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp1515757404449/key/foreign-keysref-type nameOnline Database45/ref-typecontributorsauthorsauthorNaidoo, B/author/authors/contributorstitlestitleSouth Africa pushes ahead with carbon dioxide storage Atlas project, but scepticism persists/titlesecondary-titleEngineering News/secondary-title/titlesedition16 January 2009/editiondatesyear2009/yearpub-datesdate19 July 2012/date/pub-dates/datesurlsrelated-urlsurlhttp//www.engineeringnews.co.za/article/south-africa-pushes-ahead-with-carbon-dioxide-storage-atlas-project-but-scepticism-persists-2009-01-16/url/related-urls/urls/record/Cite/EndNote6. Since acceding to the Kyoto Protocol in Copenhagen in 2009, South Africa has committed to cut GHG emissions by at least 34 by 2020 and 42 by 2025 subject to receiving sufficient financial support as well as necessary technology from international fraternity HYPERLINK l _ENREF_7 o Mabuza, 2015 450 ADDIN EN.CITE EndNoteCiteAuthorMabuza/AuthorYear2015/YearRecNum450/RecNumDisplayTextstyle facesuperscript7/style/DisplayTextrecordrec-number450/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp1515757404450/key/foreign-keysref-type nameConference Proceedings10/ref-typecontributorsauthorsauthorMabuza, Major, M,/authorauthorPremlall, Kasturie/author/authors/contributorstitlestitlestyle facenormal fontdefault size100Sorption of Industrial Flues Gases on South African Coals for CO/stylestyle facesubscript fontdefault size1002/stylestyle facenormal fontdefault size100 Storage Experimental Study on Laboratory Scal/style/titlesecondary-titlestyle facenormal fontdefault size1003/stylestyle facesuperscript fontdefault size100rd/stylestyle facenormal fontdefault size100 African Public Officials Energy and Environment Conference amp Workshop 2015/style/secondary-title/titlespages15-21/pagesdatesyear2015/year/datespub-locationCenturion, Pretoria, South Africa/pub-locationpublisherTshwane University of Technology/publisherisbn978-0-620-65945-1/isbnurls/urls/record/Cite/EndNote7. Carbon capture and storage technologies (CCS) is one of the integral parts of the Intergovernmental Panel on Climate Change (IPCC) HYPERLINK l _ENREF_8 o IPCC, 2014 446 ADDIN EN.CITE EndNoteCite ExcludeAuth1AuthorIPCC/AuthorYear2014/YearRecNum446/RecNumDisplayTextstyle facesuperscript8/style/DisplayTextrecordrec-number446/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp1515757404446/key/foreign-keysref-type nameReport27/ref-typecontributorsauthorsauthorIPCC/author/authorssecondary-authorsauthorEdenhofer, O/authorauthorPichs-Madruga, R/authorauthorSokona, Y/authorauthorFarahani, E/authorauthorKadner, S/authorauthorSeyboth, K/authorauthorAdler, A/authorauthorBaum, I/authorauthorBrunner, S/authorauthorEichemeier, P/authorauthorKriemann, B/authorauthorSavolainen, J/authorauthorSchlmer, S/authorauthorvon Stechow, C/authorauthorZwickel, T/authorauthorMinx, J, C/author/secondary-authors/contributorstitlestitleSummary for policymakers/titlesecondary-titleClimate Change 2014 Mitigation Climate Change Contribution of Working Group III to the Fifth Assessment Report of the Intergovernmental panel on Climate Change/secondary-title/titlesnum-volsCambridge University Press/num-volsdatesyear2014/year/datespub-locationCambridge, UK and New York, New York, USA/pub-locationurls/urls/record/Cite/EndNote8 strategies to reduce the amount of CO2 in the atmosphere HYPERLINK l _ENREF_9 o de_Richter, 2016 443 ADDIN EN.CITE EndNoteCiteAuthorde_Richter/AuthorYear2016/YearRecNum443/RecNumDisplayTextstyle facesuperscript9/style/DisplayTextrecordrec-number443/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp1515757404443/key/foreign-keysref-type nameJournal Article17/ref-typecontributorsauthorsauthorde_Richter, Renaud K./authorauthorMing, Tingzhen/authorauthorCaillol, Sylvain/authorauthorLiu, Wei/author/authors/contributorstitlestitleFighting global warming by GHG removal Destroying CFCs and HCFCs in solar-wind power plant hybrids producing renewable energy with no-intermittency/titlesecondary-titleInternational Journal of Greenhouse Gas Control/secondary-title/titlesperiodicalfull-titleInternational Journal of Greenhouse Gas Control/full-title/periodicalpages449-472/pagesvolume49/volumekeywordskeywordPhotocatalytic oxydo-reduction/keywordkeywordGreenhouse gases removal/keywordkeywordClimate forcers elimination/keywordkeywordGlobal warming reduction/keywordkeywordSolar updraft chimney power plant/keywordkeywordCO2-free renewable energy/keywordkeywordNegative emissions technology/keyword/keywordsdatesyear2016/year/datesisbn1750-5836/isbnurlsrelated-urlsurlhttp//www.sciencedirect.com/science/article/pii/S1750583616300858/url/related-urls/urlselectronic-resource-numhttp//dx.doi.org/10.1016/j.ijggc.2016.02.027/electronic-resource-num/record/Cite/EndNote9. Due to the growing awareness of the importance of CCS in resolving global warming issues, enormous efforts have been made in the political sphere, engineering and academic sectors to extend our knowledge and role of this technology HYPERLINK l _ENREF_10 o Zhang, 2009 324 ADDIN EN.CITE EndNoteCiteAuthorZhang/AuthorYear2009/YearRecNum324/RecNumDisplayTextstyle facesuperscript10/style/DisplayTextrecordrec-number324/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp1515757213324/key/foreign-keysref-type nameJournal Article17/ref-typecontributorsauthorsauthorZhang, Jun/authorauthorXiao, Penny/authorauthorLi, Gang/authorauthorWebley, Paul A./author/authors/contributorstitlestitleEffect of flue gas impurities on CO2 capture performance from flue gas at coal-fired power stations by vacuum swing adsorption/titlesecondary-titleEnergy Procedia/secondary-title/titlesperiodicalfull-titleEnergy Procedia/full-title/periodicalpages1115-1122/pagesvolume1/volumenumber1/numberkeywordskeywordCarbon dioxide capture/keywordkeywordFlue gas/keywordkeywordVacuum swing adsorption/keywordkeywordImpurity/keyword/keywordsdatesyear2009/year/datesisbn1876-6102/isbnurlsrelated-urlsurlhttp//www.sciencedirect.com/science/article/pii/S1876610209001489/url/related-urls/urlselectronic-resource-numhttp//dx.doi.org/10.1016/j.egypro.2009.01.147/electronic-resource-num/record/Cite/EndNote10. In 2010, the South African Centre for Carbon Capture and Storage (SACCCS) launched an atlas on geological storage of CO2 of South Africa, this was succeeded by a full report on the same survey to identify potential storage sites and their respective storage capacities for South Africa ADDIN EN.CITE EndNoteCiteAuthorCloete/AuthorYear2010/YearRecNum451/RecNumDisplayTextstyle facesuperscript11, 12/style/DisplayTextrecordrec-number451/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp1515757404451/key/foreign-keysref-type nameReport27/ref-typecontributorsauthorsauthorCloete, M/author/authorstertiary-authorsauthorCouncil for Geoscience/author/tertiary-authors/contributorstitlestitleAtlas on geological storage of carbon dioxide in South Africa/title/titlespages1-59/pagesdatesyear2010/year/datespub-locationSilverton, Pretoria, South Africa/pub-locationpublisherCouncil for Geoscience/publisherisbnISBN978-1-920226-24-4/isbnurls/urls/record/CiteCiteAuthorViljoen/AuthorYear2010/YearRecNum325/RecNumrecordrec-number325/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp1515757213325/key/foreign-keysref-type nameReport27/ref-typecontributorsauthorsauthorViljoen, J, H, A/authorauthorStapelberg, F, D, J/authorauthorCloete, M/author/authorssecondary-authorsauthorDownes, G/authorauthorvan der Spuy, D/authorauthorvan Eck, S/authorauthorvan Heerden, A/author/secondary-authors/contributorstitlestitleTechnical Report on th Geological Storage of Carbon Dioxide in South Africa/title/titlesdatesyear2010/year/datespub-locationSilverton Pretoria/pub-locationpublisherCouncil for Geoscience/publisherurls/urls/record/Cite/EndNote HYPERLINK l _ENREF_11 o Cloete, 2010 451 11, HYPERLINK l _ENREF_12 o Viljoen, 2010 325 12. The survey showed that there is an overall CO2 storage potential of 150 gigatonnes (Gt), for which 1271.9 million tonnes (Mt) is in the coal fields. Injection of CO2 into unmineable coal seams is considerably one of the most attractive systems to sequester CO2 however, precise knowledge of injection and sorption-induced coal property changes are essential for safe and successful implementation of this storage technique HYPERLINK l _ENREF_13 o Ranathunga, 2016 14 ADDIN EN.CITE EndNoteCiteAuthorRanathunga/AuthorYear2016/YearRecNum14/RecNumDisplayTextstyle facesuperscript13/style/DisplayTextrecordrec-number14/rec-numberforeign-keyskey appEN db-id9vtzasfz8sx2tjessax5td9a2rv2dsvrfdvp14/key/foreign-keysref-type nameJournal Article17/ref-typecontributorsauthorsauthorRanathunga, A. S./authorauthorPerera, M. S. A./authorauthorRanjith, P. G./author/authors/contributorstitlestitlestyle facenormal fontdefault size100Influence of CO/stylestyle facesubscript fontdefault size1002/stylestyle facenormal fontdefault size100 adsorption on the strength and elastic modulus of low rank Australian coal under confining pressure/style/titlesecondary-titleInternational Journal of Coal Geology/secondary-title/titlesperiodicalfull-titleInternational Journal of Coal Geology/full-title/periodicalkeywordskeywordCO2 adsorption/keywordkeywordStrength and elastic modulus/keywordkeywordCO2 phase and pressure/keywordkeywordCoal rank/keywordkeywordStress environment/keyword/keywordsdatesyear2016/year/datesisbn0166-5162/isbnurlsrelated-urlsurlhttp//www.sciencedirect.com/science/article/pii/S0166516216302087/url/related-urls/urlselectronic-resource-numhttp//dx.doi.org/10.1016/j.coal.2016.08.027/electronic-resource-num/record/Cite/EndNote13. Injecting CO2 into unmineable coal seams consists of two beneficial parts i.e. of enhanced coalbed methane recovery and CO2 sequestration. In conventional geological reservoirs, CO2 is proclaimed to be trapped by four mechanisms including capillary or residual, structural, mineral and dissolution trappings. However, adsorption trapping of CO2 is the most dominant storage mechanism in coal matrix HYPERLINK l _ENREF_14 o Arif, 2016 453 ADDIN EN.CITE EndNoteCiteAuthorArif/AuthorYear2016/YearRecNum453/RecNumDisplayTextstyle facesuperscript14/style/DisplayTextrecordrec-number453/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp1515757404453/key/foreign-keysref-type nameJournal Article17/ref-typecontributorsauthorsauthorArif, Muhammad/authorauthorBarifcani, Ahmed/authorauthorLebedev, Maxim/authorauthorIglauer, Stefan/author/authors/contributorstitlestitlestyle facenormal fontdefault size100CO/stylestyle facesubscript fontdefault size1002/stylestyle facenormal fontdefault size100-wettability of low to high rank coal seams Implications for carbon sequestration and enhanced methane recovery/style/titlesecondary-titleFuel/secondary-title/titlesperiodicalfull-titleFuel/full-title/periodicalpages680-689/pagesvolume181/volumekeywordskeywordCoal bed methane/keywordkeywordWettability/keywordkeywordRank/keywordkeywordPressure/keywordkeywordTemperature/keywordkeywordContact angle/keywordkeywordCO2 storage/keyword/keywordsdatesyear2016/year/datesisbn0016-2361/isbnurlsrelated-urlsurlhttp//www.sciencedirect.com/science/article/pii/S0016236116303684/url/related-urls/urlselectronic-resource-numhttp//dx.doi.org/10.1016/j.fuel.2016.05.053/electronic-resource-num/record/Cite/EndNote14. In the framework of geological storage of CO2 in unmineable coal seams, to date, little attention has been focused on direct injection of flue gases from power plants or other flue gas emitting sources into geological storage site such as coal seams. There is limited understanding of flue gas sorption behavior into unmineable coal seams, particularly, for South African coals HYPERLINK l _ENREF_15 o Mabuza, 2014 245 ADDIN EN.CITE EndNoteCiteAuthorMabuza/AuthorYear2014/YearRecNum245/RecNumDisplayTextstyle facesuperscript15/style/DisplayTextrecordrec-number245/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp1515757162245/key/foreign-keysref-type nameJournal Article17/ref-typecontributorsauthorsauthorMabuza, Major/authorauthorPremlall, Kasturie/author/authors/contributorstitlestitlestyle facenormal fontdefault size100Assessing Impure CO/stylestyle facesubscript fontdefault size1002/stylestyle facenormal fontdefault size100 Adsorption Capacity on Selected South African Coals Comparative Study Using Low and High Concentrated Simulated Flue Gases/style/titlesecondary-titleEnergy Procedia/secondary-title/titlesperiodicalfull-titleEnergy Procedia/full-title/periodicalpages308-315/pagesvolume51/volumekeywordskeywordCoal/keywordkeywordflue gases/keywordkeywordadsorption isotherms/keywordkeywordadsorption capacity/keyword/keywordsdatesyear2014/yearpub-datesdate2014/01/01//date/pub-dates/datesisbn1876-6102/isbnurlsrelated-urlsurlhttp//www.sciencedirect.com/science/article/pii/S1876610214008996/url/related-urls/urlselectronic-resource-numhttp//dx.doi.org/10.1016/j.egypro.2014.07.037/electronic-resource-num/record/Cite/EndNote15. Therefore, this paper presents effect of impurities in CO2 stream on CO2 sorption capacity of selected South African coals using synthetic flue gas (containing 12 CO2, 5.5 O2, 82 N2, 0.38 SO2, and 0.12 NO2) to mimic the industrial flue gas from coal-fired power plant instead of pure CO2 for experimental purposes. The sorption measurements were done under reservoir in-situ and supercritical CO2 conditions, this provided reasonable experimental basis to enable conclusive predictive assessments flue gas and CO2 sequestration. Experimental Sample description and preparation Three South African coals from at least three different coalfields located in the main Karoo basin were used in this study. These coals are from Ermelo (Coal EML), Somkhele (Coal SML), and Springlake (Coal SPL). These coals were selected based on their coal rank and coal maceral compositions and they represent major commercial coal fields in South Africa. In addition, these coalfields have been earmarked as potential future CO2 storage sites as they were mentioned by Viljoen et al. HYPERLINK l _ENREF_12 o Viljoen, 2010 325 ADDIN EN.CITE EndNoteCite ExcludeAuth1AuthorViljoen/AuthorYear2010/YearRecNum325/RecNumDisplayTextstyle facesuperscript12/style/DisplayTextrecordrec-number325/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp1515757213325/key/foreign-keysref-type nameReport27/ref-typecontributorsauthorsauthorViljoen, J, H, A/authorauthorStapelberg, F, D, J/authorauthorCloete, M/author/authorssecondary-authorsauthorDownes, G/authorauthorvan der Spuy, D/authorauthorvan Eck, S/authorauthorvan Heerden, A/author/secondary-authors/contributorstitlestitleTechnical Report on th Geological Storage of Carbon Dioxide in South Africa/title/titlesdatesyear2010/year/datespub-locationSilverton Pretoria/pub-locationpublisherCouncil for Geoscience/publisherurls/urls/record/Cite/EndNote12 as depicted in REF _Ref425351657 h MERGEFORMAT Figure 1. The CO2 storage potential for Somkhele, Ermelo, and Springlake coalfields has been estimated to be 82.9, 331.8 and 43.1 Mt, respectively. This amounts to about a third of the entire CO2 storage potential in South African coalfields. ( REF _Ref425351657 h MERGEFORMAT Figure 1) The coal samples were collected in situ using a hammer and a crow bar from respective coalfields. The samples were placed in plastics bags, which was sealed on site before transportation to our laboratory. In order to avoid excess exposure to the atmosphere and prevent oxidation, the samples were flushed with an inert nitrogen gas and then stored in a refrigerator (3 C temperature condition). 2.2. CO2 sorption experiments A high-pressure volumetric sorption system (HPVSS) was designed, constructed and commissioned to conduct to estimate the flue gas and CO2 sorption capacity on the coal samples studied. A schematic of the HPVSS is shown in REF _Ref464485046 h MERGEFORMAT Figure 2. ( REF _Ref464485046 h MERGEFORMAT Figure 2) The experimental setup consists of a sample drying vessel, reactor cell, reference cell and a digital control system for pressure and temperature recordings. The reference and reactor cells were manufactured of stainless steel with volumes of 467.2 cm3 and 43.79 cm3, respectively. The pressure in the reference and reactor cells was controlled and monitored by a digital control system connected to a WIKA pressure transducer (model A-10). An SRI Gas Chromatograph (GC) (Model 8610) supplied by Chromspec Chromatography is connected to the HPVSS experimental setup by a 1/8 in. stainless steel tube and was used to measure the flue gas composition before and after each sorption test. A data logging system connected to the pressure and temperature transducers was used to collect the pressure and temperature data five seconds. Pure CO2 sorption isotherms were measured at 30, 40, 50, and 60 C and at pressures up to 9.0 MPa. This temperature profile is based on the coal reservoir temperature and pressure profiles as reported by Zang HYPERLINK l _ENREF_16 o Zhang, 2008 30 ADDIN EN.CITE EndNoteCiteAuthorZhang/AuthorYear2008/YearRecNum30/RecNumDisplayTextstyle facesuperscript16/style/DisplayTextrecordrec-number30/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp151575681130/key/foreign-keysref-type nameJournal Article17/ref-typecontributorsauthorsauthorZhang, Qing-ling/author/authors/contributorstitlestitleAdsorption mechanism of different coal ranks under variable temperature and pressure conditions/titlesecondary-titleJournal of China University of Mining and Technology/secondary-title/titlesperiodicalfull-titleJournal of China University of Mining and Technology/full-title/periodicalpages395-400/pagesvolume18/volumenumber3/numberkeywordskeywordcoal/keywordkeywordvariable temperature and pressure test/keywordkeywordadsorption/keywordkeywordcharacteristics/keyword/keywordsdatesyear2008/yearpub-datesdate2008/09/01/date/pub-dates/datesisbn1006-1266/isbnurlsrelated-urlsurlhttp//www.sciencedirect.com/science/article/pii/S1006126608600838/url/related-urls/urlselectronic-resource-numhttp//dx.doi.org/10.1016/S1006-1266(08)60083-8/electronic-resource-num/record/Cite/EndNote16, with the targeted CO2 sequestration depth of 800 m and above, 30 C was, therefore, taken as the lowest temperature. Each sorption test involved eight consecutive procedures sample degassing moisture equilibrating the sample filling the reactor cell with the coal reactor cell evacuation using a vacuum pump void volume (Vvoid) determination of the reactor cell filled with a coal sample injecting CO2 into the reference cell expanding the CO2 into the reactor cell and, data recording. Each coal sample was degassed under vacuum conditions at 130 C and, subsequently, moisture equilibrated to 4 using deionized water before the sorption measurements could take place. Sorption capacity and other properties such as the density, pore size, surface area, and porosity for coals could be affected by the presence of moisture within the coal sample HYPERLINK l _ENREF_17 o Ozdemir, 2004 461 ADDIN EN.CITE EndNoteCiteAuthorOzdemir/AuthorYear2004/YearRecNum461/RecNumDisplayTextstyle facesuperscript17/style/DisplayTextrecordrec-number461/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp1515757405461/key/foreign-keysref-type nameThesis32/ref-typecontributorsauthorsauthorOzdemir, E/author/authors/contributorstitlestitlestyle facenormal fontdefault size100Chemistry of the adsorption of carbon dioxide by Argonne premium coals and a model to simulate CO/stylestyle facesubscript fontdefault size1002/stylestyle facenormal fontdefault size100 sequestration in coal seams/style/titlesecondary-titleSchool of Engineering/secondary-title/titlesvolumePhD/volumedatesyear2004/year/datespub-locationPittsburgh/pub-locationpublisherUniversity of Pittsburgh/publisherurls/urls/record/Cite/EndNote17, other elucidations cannot be precluded entirely however, residual moisture seems to play the most dominant role in affecting the sorption capacity on coals HYPERLINK l _ENREF_18 o Goodman, 2004 168 ADDIN EN.CITE EndNoteCiteAuthorGoodman/AuthorYear2004/YearRecNum168/RecNumDisplayTextstyle facesuperscript18/style/DisplayTextrecordrec-number168/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp1515756852168/key/foreign-keysref-type nameJournal Article17/ref-typecontributorsauthorsauthorGoodman, A. L./authorauthorBusch, A./authorauthorDuffy, G. J./authorauthorFitzgerald, J. E./authorauthorGasem, K. A. M./authorauthorGensterblum, Y./authorauthorKrooss, B. M./authorauthorLevy, J./authorauthorOzdemir, E./authorauthorPan, Z./authorauthorRobinson, R. L./authorauthorSchroeder, K./authorauthorSudibandriyo, M./authorauthorWhite, C. M./author/authors/contributorstitlestitlestyle facenormal fontdefault size100An Inter-laboratory Comparison of CO/stylestyle facesubscript fontdefault size1002/stylestyle facenormal fontdefault size100 Isotherms Measured on Argonne Premium Coal Samples/style/titlesecondary-titleEnergy amp Fuels/secondary-title/titlesperiodicalfull-titleEnergy amp Fuels/full-title/periodicalpages1175-1182/pagesvolume18/volumenumber4/numberdatesyear2004/yearpub-datesdate2004/07/01/date/pub-dates/datespublisherAmerican Chemical Society/publisherisbn0887-0624/isbnurlsrelated-urlsurlhttp//dx.doi.org/10.1021/ef034104h/url/related-urls/urlselectronic-resource-num10.1021/ef034104h/electronic-resource-num/record/Cite/EndNote18. Each sample was then placed inside the sample cell and, thereafter, subjected to vacuum for 15 minutes so as to evacuate the system of any former gases. The void volume (see REF _Ref464484876 h MERGEFORMAT Figure 3), Vvoid, in the sample cell was estimated using the helium expansion approach as described by Sudibandriyo HYPERLINK l _ENREF_19 o Sudibandriyo, 2010 463 ADDIN EN.CITE EndNoteCite ExcludeAuth1AuthorSudibandriyo/AuthorYear2010/YearRecNum463/RecNumDisplayTextstyle facesuperscript19/style/DisplayTextrecordrec-number463/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp1515757405463/key/foreign-keysref-type nameJournal Article17/ref-typecontributorsauthorsauthorSudibandriyo, M/author/authors/contributorstitlestitlestyle facenormal fontdefault size100A simple technique for surface area determintation through supercritical CO/stylestyle facesubscript fontdefault size1002/stylestyle facenormal fontdefault size100 adsorption/style/titlesecondary-titleMakara Seri Teknologi/secondary-title/titlesperiodicalfull-titleMakara Seri Teknologi/full-title/periodicalpages1-6/pagesvolume14/volumenumber1/numberdatesyear2010/year/datesisbn16936698/isbnurls/urls/record/Cite/EndNote19. ( REF _Ref464484876 h MERGEFORMAT Figure 3) The helium was then evacuated and the sorbate (pure CO2 or flue gas) was introduced into the system. Nine incremental pressure steps were preferred for these sorption tests and they were increased at intervals of 1.0 MPa until 9.0 MPa was reached. During the initial (trial) tests run up to 24 hours, it was discovered that 90 minutes was adequate for the equilibrium point to be reached. The recorded data of pressure and temperature was used estimate the amount of gas sorbed in millimoles of CO2 per gram of coal tested. Flue gas sorption isotherms measurements The flue gas sorption tests of CO2/O2/N2/SO2/NO2 on South African coals at 30 and 60 C, and pressures up to 9.0 MPa were conducted at 12/5.5/82/0.38/0.12 mole feed composition. For flue gas sorption isotherms measurements, the procedure was exactly similar to that of pure gas sorption isotherms measurements. The only significant distinction was that after equilibrium pressure was reached for each pressure step, the gas remaining in the gas-phase in the sample cell was sampled via the sample valve connector (connected between the reactor cell and the GC) to the gas chromatograph. This was done to determine the un-sorbed amount of each individual gas. Initially, the flue gas was sampled from the cylinder and analyzed using the GC to validate the composition of the gas as received from the supplier. Results Proximate and Petrographic Analysis REF _Ref466042013 h MERGEFORMAT Table 1 shows the maceral composition and proximate analysis of the three coals under investigation. Coal SML has high vitrinite content of 84 vol and low inertinite of 11.5 vol, Coal EML has high inertinite content of 74.2 vol with low vitrinite content of 12.8 vol, and Coal SPL has almost 50/50 vol for each of vitrinite and inertinite contents. Coal SPL will be used as a control particularly when discussing the effects of coal macerals. It should also be noted that Coal EML has significantly high mineral and volatile matters of 9.8 vol and 59.8 wt, respectively. ( REF _Ref466042013 h MERGEFORMAT Table 1) High-pressure pure CO2 sorption The sorption isotherms of high-pressure pure CO2 experiments conducted on moisture equilibrated South African coals are shown in REF _Ref464664528 h MERGEFORMAT Figure 4. These sorption experiments reached a maximum CO2 pressure of 9.0 MPa at all four temperatures at which they were conducted. All isotherms increased monotonously from low to sub-critical pressures and exhibit a monotonous asymptotic behavior at high pressures ( 6.0 MPa). This behavior was consistently observed for all the isotherms measured at all different temperatures. ( REF _Ref464664528 h MERGEFORMAT Figure 4) REF _Ref464721409 h MERGEFORMAT Table 2 summarizes all the CO2 sorption capacities at all the 4 temperatures investigated in this study. At the final pressures of the sorption isotherms in REF _Ref464664528 h MERGEFORMAT Figure 4, the sorption capacity of CO2 was determined to range from 2.25 4.16 mmol CO2/g coal (0.099 0.183 tons of CO2 per ton of coal). The highest sorption capacities were observed at 30 C with maximum sorption capacity ranging from 3.46 4.16 mmol CO2/g coal (0.152 0.183 tons of CO2 per ton of coal). Furthermore, Coal SML consistently displayed the highest sorption capacity of all the coals studied, more evidently at higher pressures ( 6.0 MPa). ( REF _Ref464721409 h MERGEFORMAT Table 2) REF _Ref464723710 h MERGEFORMAT Figure 5 compares the sorption capacities of Coal SML at different temperatures. This comparison was performed to study the effect of temperature on the high-pressure pure CO2 sorption capacity on coals. Since Coal SML was established to have the highest sorption capacities, it was in the interest of this study to use it as basis to evaluate this effect. It is observed that maximum sorption capacity consistently decreases with an increase in isothermal temperature. ( REF _Ref464723710 h MERGEFORMAT Figure 5) High-pressure flue gas sorption The results of high-pressure sorption isotherms of flue gas on moisture equilibrated South African coals are shown in REF _Ref464739974 h MERGEFORMAT Figure 6 and REF _Ref504566294 h MERGEFORMAT Figure 7 together with sorption capacity of each component of the flue gas. REF _Ref464739974 h MERGEFORMAT Figure 6 and REF _Ref504566294 h MERGEFORMAT Figure 7 also present preferential sorption results of the individual gases on coals. As was the case for pure CO2, these sorption experiments reached a maximum flue gas pressure of 9.0 MPa however, results of sorption experiments conducted at temperatures of 30 and 60 C are presented. Furthermore, the feed composition used was 12CO2/5.5O2/82N2/0.38 SO2/0.12NO2. The total flue gas sorption capacity on the coals ranges from 2.34 3.96 mmol CO2/g-coal (0.081 0.128 tons CO2 per ton of coal). ( REF _Ref464739974 h MERGEFORMAT Figure 6) ( REF _Ref504566294 h MERGEFORMAT Figure 7) In REF _Ref464739974 h MERGEFORMAT Figure 6 and REF _Ref504566294 h MERGEFORMAT Figure 7, it is observed that the the sorption capacity of each component increases with an increase in gas pressure. All isotherms consistently exhibit a monotonous increasing trend until the final pressure (9.0 MPa) without reaching any asymptotic stage. The O2, SO2 and NO2 trends increase very slowly with increasing pressure compared to those ones of CO2 and N2. In the current study, the approach applied by Luo et al. HYPERLINK l _ENREF_20 o Luo, 2015 459 ADDIN EN.CITE EndNoteCiteAuthorLuo/AuthorYear2015/YearRecNum459/RecNumDisplayTextstyle facesuperscript20/style/DisplayTextrecordrec-number459/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp1515757405459/key/foreign-keysref-type nameJournal Article17/ref-typecontributorsauthorsauthorLuo, Xiangrong/authorauthorWang, Shuzhong/authorauthorWang, Zhiguo/authorauthorJing, Zefeng/authorauthorLv, Mingming/authorauthorZhai, Zhende/authorauthorHan, Tao/author/authors/contributorstitlestitleAdsorption of methane, carbon dioxide and their binary mixtures on Jurassic shale from the Qaidam Basin in China/titlesecondary-titleInternational Journal of Coal Geology/secondary-title/titlesperiodicalfull-titleInternational Journal of Coal Geology/full-title/periodicalpages210-223/pagesvolume150151/volumekeywordskeywordShale gas/keywordkeywordPreferential adsorption/keywordkeywordPore structure/keywordkeywordIsosteric heat of adsorption/keyword/keywordsdatesyear2015/year/datesisbn0166-5162/isbnurlsrelated-urlsurlhttp//www.sciencedirect.com/science/article/pii/S0166516215300501/url/related-urls/urlselectronic-resource-numhttp//dx.doi.org/10.1016/j.coal.2015.09.004/electronic-resource-num/record/Cite/EndNote20 to assess selective sorption of CO2 and CH4 gases on Jurassic shale from the Qaidam Basin in China was adopted for the assessment of the occurrence of preferential sorption of CO2, N2, O2, SO2 and NO2 gases on moisture equilibrated South African coals. From both REF _Ref464739974 h MERGEFORMAT Figure 6 and REF _Ref504566294 h MERGEFORMAT Figure 7, all coal samples reveal a preferential CO2 sorption trend at both 30 and 60 C with the exception of Coal SPL ( REF _Ref464739974 h MERGEFORMAT Figure 6 (c)) which exhibit a slight (non-significant) preferential N2 sorption trend at 30 C. This (Coal SPL trend) is more evident at high pressures (subcritical to supercritical). REF _Ref464746612 h MERGEFORMAT Table 3 shows results of total gas (including all gases) and CO2 sorption capacity when flue gas was injected into the three coal samples at 30 C. The CO2 sorption capacities calculated from experimental data range from 1.30 1.55 mmol CO2/g-coal (0.054 0.068 tons of CO2 per ton of coal), and the total gas sorption capacity range from 3.38 3.96 mmol gas/g-coal. As with pure CO2 injection, Coal SML is observed to have the highest for both total gas and CO2 sorption capacities of 3.96 mmol gas/g-coal and 1.55 mmol CO2/g-coal, respectively. Coal EML has the lowest sorption capacities of 3.38 mmol gas/g-coal and 1.41 mmol CO2/g-coal, this trend was also observed for pure CO2 injection. ( REF _Ref464746612 h MERGEFORMAT Table 3) Comparison of CO2 sorption capacities for pure CO2 and flue gas injection REF _Ref464749619 h MERGEFORMAT Figure 8 compares sorption capacities for pure CO2 and flue gas on Coal SML. Coal SML was used as basis to perform this comparison due its consistent nature of high sorption capacity as discovered in this study. However, same trends were obtained for the other two coals (EML and SPL). CO2 sorption capacity was significantly higher when pure CO2 was injected than when flue gas was injected into the coal under similar conditions of temperature and pressure. This difference was calculated to be 63 on average. ( REF _Ref464749619 h MERGEFORMAT Figure 8) In the context of total gas uptake, presented in REF _Ref464751941 h MERGEFORMAT Figure 9, the maximum amount of gas that could be sorbed by Coal SML at 30 C and pressures up 9.0 MPa was 4.16 (0.183 tonne of CO2 per tonne of coal) and 3.96 mmol gas/g-coal (0.123 tonne of gas per tonne of coal) for pure CO2 and flue gas, respectively. The difference was calculated to be 5 in mole basis (30 mass basis). ( REF _Ref464751941 h MERGEFORMAT Figure 9) Discussion Proximate and Petrographic Analysis As mentioned in section REF _Ref466030686 n h MERGEFORMAT 3.1, Coal SML has high carbon content with low volatile and mineral matter contents this makes it more favourable for sorption of CO2. According to Beamish et al. HYPERLINK l _ENREF_21 o Beamish, 1998 478 ADDIN EN.CITE EndNoteCite ExcludeAuth1AuthorBeamish/AuthorYear1998/YearRecNum478/RecNumDisplayTextstyle facesuperscript21/style/DisplayTextrecordrec-number478/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp1515757405478/key/foreign-keysref-type nameConference Paper47/ref-typecontributorsauthorsauthorBeamish, B/authorauthorLaxminarayana, C/authorauthorCrosdale, P, J/author/authors/contributorstitlestitleContrasts in Methane Sorption Properties Between New Zealand and Australian coals/titlesecondary-titleCoal Operationsapos Conference/secondary-title/titlespages561-565/pagesdatesyear1998/yearpub-datesdate18 February/date/pub-dates/datespub-locationUniversity of Wollongong/pub-locationpublisherUniversity of Wollongong amp the Australian Institute of Mining and Metallurgy/publisherurlsrelated-urlsurlhttp//ro.uow.edu.au/cgi/viewcontent.cgiarticle1224ampcontextcoal/url/related-urls/urlsaccess-date16 October 2012/access-date/record/Cite/EndNote21 microporosity in coals is decreased by the existence of volatile constituents which block the micropore structure. This means that the lower the volatile matter present in coal the less micropore structure blockages for CO2 sorption. Effects of coal maceral composition A common trend was observed for the CO2 sorption capacities of the three coals studied. CO2 sorption capacities increased with an increase in vitrinite content up to pressures of 9.0 MPa and temperatures up to 60 C. This trend is in line with the observations made by Clarkson and Bustin HYPERLINK l _ENREF_22 o Clarkson, 1996 103 ADDIN EN.CITE EndNoteCite ExcludeAuth1AuthorClarkson/AuthorYear1996/YearRecNum103/RecNumDisplayTextstyle facesuperscript22/style/DisplayTextrecordrec-number103/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp1515756832103/key/foreign-keysref-type nameJournal Article17/ref-typecontributorsauthorsauthorClarkson, Christopher R./authorauthorBustin, Marc R./author/authors/contributorstitlestitleVariation in micropore capacity and size distribution with composition in bituminous coal of the Western Canadian Sedimentary Basin/titlesecondary-titleFuel/secondary-title/titlesperiodicalfull-titleFuel/full-title/periodicalpages1483-1498/pagesvolume75/volumenumber13/numberkeywordskeywordcoal/keywordkeywordmicropore structure/keywordkeywordpetrography/keyword/keywordsdatesyear1996/yearpub-datesdate1996/10/01/date/pub-dates/datesisbn0016-2361/isbnurlsrelated-urlsurlhttp//www.sciencedirect.com/science/article/pii/0016236196001421/url/related-urls/urlselectronic-resource-numhttp//dx.doi.org/10.1016/0016-2361(96)00142-1/electronic-resource-num/record/Cite/EndNote22 and was also reported by Maphala HYPERLINK l _ENREF_23 o Maphala, 2012 32 ADDIN EN.CITE EndNoteCite ExcludeAuth1AuthorMaphala/AuthorYear2012/YearRecNum32/RecNumDisplayTextstyle facesuperscript23/style/DisplayTextrecordrec-number32/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp151575681232/key/foreign-keysref-type nameThesis32/ref-typecontributorsauthorsauthorMaphala, T/author/authors/contributorstitlestitleEffects of Carbon Dioxide Storage in Coal on the Physical and Chemical Properties of Coal/titlesecondary-titleSchool of Chemical amp Metallurgical Engineering/secondary-title/titlespages240/pagesvolumeDoctor of Philosophy Degree/volumedatesyear2012/year/datespub-locationJohannesburg, South Africa/pub-locationpublisherUniversity of the Witwatersrand/publisherurls/urls/record/Cite/EndNote23. In an early study by Clarkson and Bustin HYPERLINK l _ENREF_22 o Clarkson, 1996 103 ADDIN EN.CITE EndNoteCite ExcludeAuth1AuthorClarkson/AuthorYear1996/YearRecNum103/RecNumDisplayTextstyle facesuperscript22/style/DisplayTextrecordrec-number103/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp1515756832103/key/foreign-keysref-type nameJournal Article17/ref-typecontributorsauthorsauthorClarkson, Christopher R./authorauthorBustin, Marc R./author/authors/contributorstitlestitleVariation in micropore capacity and size distribution with composition in bituminous coal of the Western Canadian Sedimentary Basin/titlesecondary-titleFuel/secondary-title/titlesperiodicalfull-titleFuel/full-title/periodicalpages1483-1498/pagesvolume75/volumenumber13/numberkeywordskeywordcoal/keywordkeywordmicropore structure/keywordkeywordpetrography/keyword/keywordsdatesyear1996/yearpub-datesdate1996/10/01/date/pub-dates/datesisbn0016-2361/isbnurlsrelated-urlsurlhttp//www.sciencedirect.com/science/article/pii/0016236196001421/url/related-urls/urlselectronic-resource-numhttp//dx.doi.org/10.1016/0016-2361(96)00142-1/electronic-resource-num/record/Cite/EndNote22 on Western Canadian Cretaceous coals, they found an increase in CO2 sorption capacities was subject to an increase in vitrinite content of the coal and it was concluded that the pore structure and GSC is essentially influenced by the coal composition. Recently, Maphala HYPERLINK l _ENREF_23 o Maphala, 2012 32 ADDIN EN.CITE EndNoteCite ExcludeAuth1AuthorMaphala/AuthorYear2012/YearRecNum32/RecNumDisplayTextstyle facesuperscript23/style/DisplayTextrecordrec-number32/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp151575681232/key/foreign-keysref-type nameThesis32/ref-typecontributorsauthorsauthorMaphala, T/author/authors/contributorstitlestitleEffects of Carbon Dioxide Storage in Coal on the Physical and Chemical Properties of Coal/titlesecondary-titleSchool of Chemical amp Metallurgical Engineering/secondary-title/titlespages240/pagesvolumeDoctor of Philosophy Degree/volumedatesyear2012/year/datespub-locationJohannesburg, South Africa/pub-locationpublisherUniversity of the Witwatersrand/publisherurls/urls/record/Cite/EndNote23 performed long-term CO2 sorption measurements on inertinite rich and vitrinite rich South African coals, and it was concluded that CO2-coal interaction is dependent on maceral composition of the coal, whereby a vitrinite rich coal has stronger CO2-coal interaction than inertinite-rich coal. Vitrinite maceral mainly contains micropores and inertinite predominantly contains macropores and mesopores HYPERLINK l _ENREF_24 o Flores, 2014 19 ADDIN EN.CITE EndNoteCiteAuthorFlores/AuthorYear2014/YearRecNum19/RecNumDisplayTextstyle facesuperscript24/style/DisplayTextrecordrec-number19/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp151575680819/key/foreign-keysref-type nameElectronic Book44/ref-typecontributorsauthorsauthorFlores, R, M/author/authors/contributorstitlestitleCoal and Coalbed Gas Fueling the Future/title/titlesdatesyear2014/yearpub-datesdate26 January 2015/date/pub-dates/datespub-locationWaltham, Massachusetts, USA/pub-locationpublisherElsevier lnc/publisherisbn9780123969729/isbnurlsrelated-urlsurlhttps//books.google.co.za/booksidF3otuH4Ld2QCamppgPA274amplpg/url/related-urls/urls/record/Cite/EndNote24 HYPERLINK l _ENREF_26 o Flores, 2014 32 . Due to its abundant microporosity, which results in high coal total pore area, vitrinite content is classified as the single most significant maceral composition in gas sequestration studies HYPERLINK l _ENREF_25 o Adeboye, 2011 28 ADDIN EN.CITE EndNoteCiteAuthorAdeboye/AuthorYear2011/YearRecNum28/RecNumDisplayTextstyle facesuperscript25/style/DisplayTextrecordrec-number28/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp151575681128/key/foreign-keysref-type nameThesis32/ref-typecontributorsauthorsauthorAdeboye, O, O/author/authors/contributorstitlestitleEffects of Coal Composition and Fabric on Porosity, Sorption Capacity and Gas Flow Properties in Western Canada Sedimentary Basin Coals/titlesecondary-titleFaculty of Graduate Studies/secondary-title/titlespages180/pagesvolumeMaster of Science in Geology/volumedatesyear2011/year/datespub-locationVancouver, British Columbia, Canada/pub-locationpublisherThe University of British Columbia/publisherurls/urls/record/Cite/EndNote25. Harris and Yust HYPERLINK l _ENREF_26 o Harris, 1976 29 ADDIN EN.CITE EndNoteCite ExcludeAuth1AuthorHarris/AuthorYear1976/YearRecNum29/RecNumDisplayTextstyle facesuperscript26/style/DisplayTextrecordrec-number29/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp151575681129/key/foreign-keysref-type nameJournal Article17/ref-typecontributorsauthorsauthorHarris, Lawrence A./authorauthorYust, Charles S./author/authors/contributorstitlestitleTransmission electron microscope observations of porosity in coal/titlesecondary-titleFuel/secondary-title/titlesperiodicalfull-titleFuel/full-title/periodicalpages233-236/pagesvolume55/volumenumber3/numberdatesyear1976/year/datesisbn0016-2361/isbnurlsrelated-urlsurlhttp//www.sciencedirect.com/science/article/pii/0016236176900946/url/related-urls/urlselectronic-resource-numhttp//dx.doi.org/10.1016/0016-2361(76)90094-6/electronic-resource-num/record/Cite/EndNote26 linked the microscopic composition of coals to porosity and pore size. This concludes that vitrinite contains numerous sorption sites compared to inertinite and liptinite. According to Crosdale et al. HYPERLINK l _ENREF_27 o Crosdale, 1998 71 ADDIN EN.CITE EndNoteCite ExcludeAuth1AuthorCrosdale/AuthorYear1998/YearRecNum71/RecNumDisplayTextstyle facesuperscript27/style/DisplayTextrecordrec-number71/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp151575682371/key/foreign-keysref-type nameJournal Article17/ref-typecontributorsauthorsauthorCrosdale, Peter J./authorauthorBeamish, B. Basil/authorauthorValix, Marjorie/author/authors/contributorstitlestitleCoalbed methane sorption related to coal composition/titlesecondary-titleInternational Journal of Coal Geology/secondary-title/titlesperiodicalfull-titleInternational Journal of Coal Geology/full-title/periodicalpages147-158/pagesvolume35/volumenumber14/numberkeywordskeywordadsorption isotherm/keywordkeywordbidisperse pore model/keywordkeyworddesorption rate/keywordkeywordmaceral composition/keywordkeywordmethane/keyword/keywordsdatesyear1998/year/datesisbn0166-5162/isbnurlsrelated-urlsurlhttp//www.sciencedirect.com/science/article/pii/S0166516297000153/url/related-urls/urlselectronic-resource-numhttp//dx.doi.org/10.1016/S0166-5162(97)00015-3/electronic-resource-num/record/Cite/EndNote27, the variation in CO2 sorption capacity are linked to pore structure development, mainly micropores, which are dependent on the coal type and rank. Furthermore, Busch et al. HYPERLINK l _ENREF_28 o Busch, 2003 169 ADDIN EN.CITE EndNoteCite ExcludeAuth1AuthorBusch/AuthorYear2003/YearRecNum169/RecNumDisplayTextstyle facesuperscript28/style/DisplayTextrecordrec-number169/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp1515756853169/key/foreign-keysref-type nameJournal Article17/ref-typecontributorsauthorsauthorBusch, Andreas/authorauthorGensterblum, Yves/authorauthorKrooss, Bernhard M./author/authors/contributorstitlestitlestyle facenormal fontdefault size100Methane and CO/stylestyle facesubscript fontdefault size1002/stylestyle facenormal fontdefault size100 sorption and desorption measurements on dry Argonne premium coals pure components and mixtures/style/titlesecondary-titleInternational Journal of Coal Geology/secondary-title/titlesperiodicalfull-titleInternational Journal of Coal Geology/full-title/periodicalpages205-224/pagesvolume55/volumenumber24/numberkeywordskeywordPreferential sorption/keywordkeywordHigh-pressure excess sorption/keywordkeywordCO2 storage/keywordkeywordCoalbed methane/keywordkeywordArgonne premium coals/keyword/keywordsdatesyear2003/year/datesisbn0166-5162/isbnurlsrelated-urlsurlhttp//www.sciencedirect.com/science/article/pii/S0166516203001137/url/related-urls/urlselectronic-resource-numhttp//dx.doi.org/10.1016/S0166-5162(03)00113-7/electronic-resource-num/record/Cite/EndNote28 ascribe an increase in the crystalline phase in the coal to an increase in CO2 sorption capacity. The increase in the crystalline phase indicates a dramatic decrease in the amount of the volatile matter, and consequently resulting in an increase in vitrinite reflectance. It is noteworthy that the effect of maceral composition on gas sorption capacity (GSC) is still a matter of argument. Even though there is currently unfound grounds of the role of coal type (especially the maceral composition) on gas sorption capacity and behavior, many researchers in this field ADDIN EN.CITE ADDIN EN.CITE.DATA HYPERLINK l _ENREF_22 o Clarkson, 1996 103 22, HYPERLINK l _ENREF_23 o Maphala, 2012 32 23, HYPERLINK l _ENREF_29 o Bhebhe, 2008 102 29-33 have speculated that coal maceral composition influences the GSC of coal HYPERLINK l _ENREF_34 o Krooss, 2002 456 ADDIN EN.CITE EndNoteCiteAuthorKrooss/AuthorYear2002/YearRecNum456/RecNumDisplayTextstyle facesuperscript34/style/DisplayTextrecordrec-number456/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp1515757405456/key/foreign-keysref-type nameJournal Article17/ref-typecontributorsauthorsauthorKrooss, B. M./authorauthorvan Bergen, F./authorauthorGensterblum, Y./authorauthorSiemons, N./authorauthorPagnier, H. J. M./authorauthorDavid, P./author/authors/contributorstitlestitleHigh-pressure methane and carbon dioxide adsorption on dry and moisture-equilibrated Pennsylvanian coals/titlesecondary-titleInternational Journal of Coal Geology/secondary-title/titlesperiodicalfull-titleInternational Journal of Coal Geology/full-title/periodicalpages69-92/pagesvolume51/volumenumber2/numberkeywordskeywordHigh-pressure adsorption/keywordkeywordExcess sorption capacity/keywordkeywordCoalbed methane/keywordkeywordCarbon dioxide/keywordkeywordPennsylvanian coals/keywordkeywordCO2 storage/keyword/keywordsdatesyear2002/year/datesisbn0166-5162/isbnurlsrelated-urlsurlhttp//www.sciencedirect.com/science/article/pii/S0166516202000782/url/related-urls/urlselectronic-resource-numhttp//dx.doi.org/10.1016/S0166-5162(02)00078-2/electronic-resource-numaccess-date20 October 2016/access-date/record/Cite/EndNote34. Effects pressure and temperature ( REF _Ref464830052 h MERGEFORMAT Figure 10) The results obtained in this study provide a distinct unfavorable effect of temperature on gas sorption capacity of coals up to pressures of 9.0 MPa. These are in complete agreement to those reported in previous studies in this area ADDIN EN.CITE ADDIN EN.CITE.DATA HYPERLINK l _ENREF_34 o Krooss, 2002 456 34, HYPERLINK l _ENREF_36 o Bustin, 1998 70 36, HYPERLINK l _ENREF_37 o Levy, 1997 72 37. According to Krooss et al. HYPERLINK l _ENREF_34 o Krooss, 2002 456 ADDIN EN.CITE EndNoteCite ExcludeAuth1AuthorKrooss/AuthorYear2002/YearRecNum456/RecNumDisplayTextstyle facesuperscript34/style/DisplayTextrecordrec-number456/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp1515757405456/key/foreign-keysref-type nameJournal Article17/ref-typecontributorsauthorsauthorKrooss, B. M./authorauthorvan Bergen, F./authorauthorGensterblum, Y./authorauthorSiemons, N./authorauthorPagnier, H. J. M./authorauthorDavid, P./author/authors/contributorstitlestitleHigh-pressure methane and carbon dioxide adsorption on dry and moisture-equilibrated Pennsylvanian coals/titlesecondary-titleInternational Journal of Coal Geology/secondary-title/titlesperiodicalfull-titleInternational Journal of Coal Geology/full-title/periodicalpages69-92/pagesvolume51/volumenumber2/numberkeywordskeywordHigh-pressure adsorption/keywordkeywordExcess sorption capacity/keywordkeywordCoalbed methane/keywordkeywordCarbon dioxide/keywordkeywordPennsylvanian coals/keywordkeywordCO2 storage/keyword/keywordsdatesyear2002/year/datesisbn0166-5162/isbnurlsrelated-urlsurlhttp//www.sciencedirect.com/science/article/pii/S0166516202000782/url/related-urls/urlselectronic-resource-numhttp//dx.doi.org/10.1016/S0166-5162(02)00078-2/electronic-resource-numaccess-date20 October 2016/access-date/record/Cite/EndNote34, this negative effect is attributed to the fact that the sorbed phase volume decrease with increasing temperature as shown in REF _Ref464829793 h MERGEFORMAT Figure 11. Furthermore, at lower temperatures the difference in densities between free gas phase and the sorbed phase tends to be smaller (see REF _Ref464830052 h MERGEFORMAT Figure 10) and the sorption on coal is no longer justified. ( REF _Ref464829793 h MERGEFORMAT Figure 11) Preferential sorption Since the sorption capacity of pure CO2 on coals is generally higher than the sorption capacity of many flue gas impurities (including N2, CH4, SO2 etc.) thus, under competitive sorption conditions, CO2 is usually expected to be preferentially be sorbed from any CO2 containing flue gas mixture. Differences were observed in the South African coals preferential sorption behavior from flue gas at high pressures. The sorption experiments indicated strong preferential sorption of CO2 over the other gases in the mixture. However, Coal SPL deviated from this trend at low temperatures. This implies that, for this flue gas mixture, high sorption preferential for CO2 or N2 may occur depending on the pressure and temperature conditions, as well as the coal composition. Hence, the dependence of coal macerals cannot be established at this point. It is probable that the preferential sorption of CO2 on coals is more complex than initially assumed. Crosdale HYPERLINK l _ENREF_38 o Crosdale, 1999 346 ADDIN EN.CITE EndNoteCite ExcludeAuth1AuthorCrosdale/AuthorYear1999/YearRecNum346/RecNumDisplayTextstyle facesuperscript38/style/DisplayTextrecordrec-number346/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp1515757213346/key/foreign-keysref-type nameConference Proceedings10/ref-typecontributorsauthorsauthorCrosdale, Peter J./author/authors/contributorstitlestitleMixed methane/carbon dioxide sorption by coal new evidence in support of pore-filling models/titlesecondary-titleInternational Coalbed Methane Symposium/secondary-title/titlesdatesyear1999/yearpub-datesdate3 – 7 May/date/pub-dates/datespub-locationTuscaloosa, Alabama, USA/pub-locationurls/urls/record/Cite/EndNote38 showed that preferential sorption of CO2 over other gases could be due to faster diffusion rate for CO2 as compared to its counterparts. This was substantiated by Busch et al. HYPERLINK l _ENREF_28 o Busch, 2003 169 ADDIN EN.CITE EndNoteCite ExcludeAuth1AuthorBusch/AuthorYear2003/YearRecNum169/RecNumDisplayTextstyle facesuperscript28/style/DisplayTextrecordrec-number169/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp1515756853169/key/foreign-keysref-type nameJournal Article17/ref-typecontributorsauthorsauthorBusch, Andreas/authorauthorGensterblum, Yves/authorauthorKrooss, Bernhard M./author/authors/contributorstitlestitlestyle facenormal fontdefault size100Methane and CO/stylestyle facesubscript fontdefault size1002/stylestyle facenormal fontdefault size100 sorption and desorption measurements on dry Argonne premium coals pure components and mixtures/style/titlesecondary-titleInternational Journal of Coal Geology/secondary-title/titlesperiodicalfull-titleInternational Journal of Coal Geology/full-title/periodicalpages205-224/pagesvolume55/volumenumber24/numberkeywordskeywordPreferential sorption/keywordkeywordHigh-pressure excess sorption/keywordkeywordCO2 storage/keywordkeywordCoalbed methane/keywordkeywordArgonne premium coals/keyword/keywordsdatesyear2003/year/datesisbn0166-5162/isbnurlsrelated-urlsurlhttp//www.sciencedirect.com/science/article/pii/S0166516203001137/url/related-urls/urlselectronic-resource-numhttp//dx.doi.org/10.1016/S0166-5162(03)00113-7/electronic-resource-num/record/Cite/EndNote28 by proving that CO2 consistently and significantly reached sorption equilibrium faster than CH4. These findings evidently show that coals under investigation have high affinity for CO2. Furthermore, all the individual component sorption isotherms display Langmuir-type I behaviour even though a definitive asymptotic point was not attained. Implications of direct flue gas injection Since the inception of the carbon, capture and storage technology and research, a number of researchers HYPERLINK l _ENREF_39 o Chen, 2003 526 ADDIN EN.CITE ADDIN EN.CITE.DATA 39-43 have since published the costs estimate for this technology. According to Al-Juaied and Whitmore HYPERLINK l _ENREF_44 o Al-Juaied, 2009 533 ADDIN EN.CITE EndNoteCiteAuthorAl-Juaied/AuthorYear2009/YearRecNum533/RecNumDisplayTextstyle facesuperscript44/style/DisplayTextrecordrec-number533/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp1517905991533/key/foreign-keysref-type nameReport27/ref-typecontributorsauthorsauthorAl-Juaied, Mohammed, A/authorauthorWhitmore, Adam/author/authorstertiary-authorsauthorEnergy Technology Innovation Policy/author/tertiary-authors/contributorstitlestitleRealistic Costs of Carbon Capture/title/titlespages49-50/pagesdatesyear2009/year/datespublisherBelfer Center for Science and International Affairs/publisherurls/urls/record/Cite/EndNote44 in a report they published through the Belfer Center for Science and International Affairs, CCS technology is estimated to cost US120 US180 per tonne of CO2. HYPERLINK l _ENREF_43 o IPCC, 2005 530 The cost of capturing CO2 is typically the greatest cost of a CCS project due to high energy requirements HYPERLINK l _ENREF_45 o Leung, 2014 532 ADDIN EN.CITE EndNoteCiteAuthorLeung/AuthorYear2014/YearRecNum532/RecNumDisplayTextstyle facesuperscript45/style/DisplayTextrecordrec-number532/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp1517493621532/key/foreign-keysref-type nameJournal Article17/ref-typecontributorsauthorsauthorLeung, Dennis Y. C./authorauthorCaramanna, Giorgio/authorauthorMaroto-Valer, M. Mercedes/author/authors/contributorstitlestitleAn overview of current status of carbon dioxide capture and storage technologies/titlesecondary-titleRenewable and Sustainable Energy Reviews/secondary-title/titlesperiodicalfull-titleRenewable and Sustainable Energy Reviews/full-title/periodicalpages426-443/pagesvolume39/volumekeywordskeywordPost-combustion/keywordkeywordPre-combustion/keywordkeywordOxyfuel combustion/keywordkeywordCO separation/keywordkeywordTransport/keywordkeywordGeological storage/keywordkeywordLeakage and monitoring/keyword/keywordsdatesyear2014/yearpub-datesdate2014/11/01//date/pub-dates/datesisbn1364-0321/isbnurlsrelated-urlsurlhttp//www.sciencedirect.com/science/article/pii/S1364032114005450/url/related-urls/urlselectronic-resource-numhttps//doi.org/10.1016/j.rser.2014.07.093/electronic-resource-num/record/Cite/EndNote45. According to Rubin et al HYPERLINK l _ENREF_43 o Rubin, 2015 531 ADDIN EN.CITE EndNoteCiteAuthorRubin/AuthorYear2015/YearRecNum531/RecNumDisplayTextstyle facesuperscript43/style/DisplayTextrecordrec-number531/rec-numberforeign-keyskey appEN db-idap0rfe0vjrxv2xeav2ovpdxmwfere0zdvfe0 timestamp1517489654531/key/foreign-keysref-type nameJournal Article17/ref-typecontributorsauthorsauthorRubin, Edward S./authorauthorDavison, John E./authorauthorHerzog, Howard J./author/authors/contributorstitlestitlestyle facenormal fontdefault size100The cost of CO/stylestyle facesubscript fontdefault size1002/stylestyle facenormal fontdefault size100 capture and storage/style/titlesecondary-titleInternational Journal of Greenhouse Gas Control/secondary-title/titlesperiodicalfull-titleInternational Journal of Greenhouse Gas Control/full-title/periodicalpages378-400/pagesvolume40/volumekeywordskeywordCarbon capture and storage/keywordkeywordCarbon sequestration/keywordkeywordPower plant costs/keywordkeywordCCS costs/keywordkeywordEconomic analysis/keyword/keywordsdatesyear2015/yearpub-datesdate2015/09/01//date/pub-dates/datesisbn1750-5836/isbnurlsrelated-urlsurlhttp//www.sciencedirect.com/science/article/pii/S1750583615001814/url/related-urls/urlselectronic-resource-numhttps//doi.org/10.1016/j.ijggc.2015.05.018/electronic-resource-num/record/Cite/EndNote43, the CO2 capture costs range from US36 US53 per tonne of CO2 this accounts for approximately 30 of the CCS technology. These costs are expected to remain unchanged over the next several decades and are based post-combustion capture on existing supercritical pulverized-coal fired power plants using bituminous coals. In the light of the abovementioned CCS technology costs, omitting the CO2 capturing process by applying direct flue gas injection into geological formations (in this case unmineable coalfields) will enable the CCS technology to be more affordable for implementation and commercialization. For instance, this study shows that the CO2 storage potential for Somkhele, Ermelo, and Springlake coalfields are 82.9, 331.8 and 43.1 Mt, respectively. In principle, this means that up to 10.2, 37.2 and 4.741 Mt of flue gas can be stored through sorption in Coals SML, EML and SPL, respectively. CONCLUSIONS This study presented high-pressure pure CO2 and flue gas sorption on three moisture equilibrated South African coals (Coal SML, Coal SPL and Coal EML) at 30 60 C and pressures up to 9.0. A comparison on the sorption capacities was evaluated and these sorption isotherms show strong differences. Experimental results show that the CO2 sorption capacity is, on average, 37 more at lower temperatures (30 C) than at higher temperatures (60 C). CO2 sorption capacity increases with an increase in pressure until a monotonous asymptotic stage is reached from subcritical ( 6.0 MPa) to supercritical (9.0 MPa) pressures. It can be concluded that pressure and temperature are one of the major controlling factors during CO2 storage in coals. Though the effect of maceral composition of GSC on coal is still controversial, results from this study show a positive correlation between the vitrinite content of the coals and their CO2 sorption capacity. CO2 sorption capacity increased significantly with increasing coal vitrinite content All coals exhibited a high preferential sorption for CO2 for the temperature and pressure range investigated in this study. 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Proximate and Petrographic Analysis of the Coals Used Analysis TypeCoal IDCoal SMLCoal EMLCoal SPLPetrographic Analysis (vol, inc. mm)Vitrinite84.012.855.3Inertinite11.574.243.3Liptinite0.03.30.0Mineral Matter4.59.81.5Vitrinite Reflectance (Ro)2.240.643.49Proximate Analysis (wt, adb)Fixed Carbon74.127.875.0Moisture1.04.51.5Ash17.317.912.8Volatile Matter7.659.810.7adb air dried basis inc. mm including mineral matter Ro – random Table SEQ Table ARABIC 2 Summary of pure CO2 Sorption Capacities. Sorption Capacity (mmol/g)Sample IDTemperature (C)30405060Coal SML4.163.412.922.54Coal SPL3.853.182.632.37Coal EML3.463.022.782.25Reference REF _Ref464664528 h MERGEFORMAT Figure 4 (a) REF _Ref464664528 h MERGEFORMAT Figure 4 (b) REF _Ref464664528 h MERGEFORMAT Figure 4 (c) REF _Ref464664528 h MERGEFORMAT Figure 4 (d) Table SEQ Table ARABIC 3 Total Gas Sorption Capacity when injecting flue gas at 30 C. Sample IDTotal Gas Capacity (mmol/g)CO2 Sorption Capacity (mmol/g)ReferenceFCoal SML3.961.55 REF _Ref464739974 h Figure 6 (a)Coal SPL3.531.30 REF _Ref464739974 h Figure 6 (b)Coal EML3.381.41 REF _Ref464739974 h Figure 6 (c) ADDIN EN.FIGURES List of Figures Figure SEQ Figure ARABIC 1. Map Showing the Location of the South African Coalfields HYPERLINK l _ENREF_46 o Hancox, 2014 20 ADDIN EN.CITE EndNoteCiteAuthorHancox/AuthorYear2014/YearRecNum20/RecNumDisplayTextstyle facesuperscript46/style/DisplayTextrecordrec-number20/rec-numberforeign-keyskey appEN db-id9vtzasfz8sx2tjessax5td9a2rv2dsvrfdvp20/key/foreign-keysref-type nameFigure37/ref-typecontributorsauthorsauthorHancox, P. John/authorauthorGtz, Annette E./author/authors/contributorstitlestitleSouth Africaaposs coalfields A 2014 perspective/titlesecondary-titleInternational Journal of Coal Geology/secondary-title/titlesperiodicalfull-titleInternational Journal of Coal Geology/full-title/periodicalkeywordskeywordGondwana coal/keywordkeywordPermian/keywordkeywordTriassic/keywordkeywordCoalfield/keywordkeywordSouth Africa/keyword/keywordsdatesyear2014/year/datespublisherElsevier/publisherisbn0166-5162/isbnlabel1/labelurlsrelated-urlsurlhttp//www.sciencedirect.com/science/article/pii/S0166516214001438/url/related-urls/urlselectronic-resource-numhttp//dx.doi.org/10.1016/j.coal.2014.06.019/electronic-resource-num/record/Cite/EndNote46 Figure SEQ Figure ARABIC 2. Schematic of the High Pressure Volumetric Sorption System Figure SEQ Figure ARABIC 3. Focused area of the HPCVSS showing the definitions for the volumetric method for gas sorption measurements ADDIN EN.CITE ADDIN EN.CITE.DATA HYPERLINK l _ENREF_28 o Busch, 2003 169 28, HYPERLINK l _ENREF_34 o Krooss, 2002 456 34 Figure SEQ Figure ARABIC 4. Excess Sorption isotherms for pure carbon dioxide on moisture equilibrated South African coals at (a) 30 C, (b) 40 C, (c) 50 C, and (d) 60 C. Figure SEQ Figure ARABIC 5. Excess sorption isotherms for pure carbon dioxide on moisture equilibrated Somkhele coal at 30 C, 40 C, 50 C, and 60 C. Figure SEQ Figure ARABIC 6. Sorption isotherms for flue gas on moisture equilibrated at 30 C (a) Coal SML, (b) Coal EML, and (c) Coal SPL. Figure SEQ Figure ARABIC 8. Comparison of sorption capacities of pure CO2 and flue gas at 30 C for moisture equilibrated Coal SML. Figure SEQ Figure ARABIC 9. Comparison of total gas uptake for Coal SML at 30 C for pure CO2 and flue gas. Figure SEQ Figure ARABIC 10. Carbon dioxide free gas and sorbed phase density profile at 30 and 60 C. Figure SEQ Figure ARABIC 11. Carbon dioxide free gas volume profile at 30 and 60 C. 1zugEnc4QDvmgzg2Y4/DD/.qHlrHrIHHkcb1xKJp([email protected] 8 NXm(Jm62n(orZB)XmxKJ IAQRAlkK4,Ee, X
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